XUV Pump-Probe Experiments on Diatomic Molecules: Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay by Kirsten SchnorrXUV Pump-Probe Experiments on Diatomic Molecules: Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay by Kirsten Schnorr

XUV Pump-Probe Experiments on Diatomic Molecules: Tracing the Dynamics of Electron Rearrangement…

byKirsten Schnorr

Hardcover | January 15, 2015

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This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy.
Title:XUV Pump-Probe Experiments on Diatomic Molecules: Tracing the Dynamics of Electron Rearrangement…Format:HardcoverDimensions:191 pagesPublished:January 15, 2015Publisher:Springer-Verlag/Sci-Tech/TradeLanguage:English

The following ISBNs are associated with this title:

ISBN - 10:3319121383

ISBN - 13:9783319121383

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Table of Contents

Introduction.- Photoionization and Interatomic Coulombic Decay.- Free-Electron Lasers.- Experimental Setup.- Data Analysis.- Ionization Dynamics of I2in XUV and IR Laser Pulses.- ICD Lifetime in Ne2.- Conclusions and Outlook.- Appendices.